壳聚糖及其衍生物去除水中汞的研究进展
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摘要
文章简介了汞离子作为一种有毒重金属在水中的危害,分析了壳聚糖作为一种生物吸附剂的结构、理化性质、改性机理和吸附机理;简要概述了以壳聚糖为基础的各种壳聚糖基吸附材料对水中有毒重金属汞离子的去除,并在此基础上简要分析了壳聚糖基吸附材料的优缺点。
The harm of mercury ion as a toxic heavy metal in water was briefly introduced. The structure, physicochemical properties, modification mechanism and adsorption mechanism of chitosan as a biological adsorbent were analyzed. The removal of toxic heavy metal mercury ions from water by various chitosan-based adsorbents was briefly summarized. On this basis, the advantages and disadvantages of chitosan-based adsorbents were briefly analyzed.
The harm of mercury ion as a toxic heavy metal in water was briefly introduced. The structure, physicochemical properties, modification mechanism and adsorption mechanism of chitosan as a biological adsorbent were analyzed. The removal of toxic heavy metal mercury ions from water by various chitosan-based adsorbents was briefly summarized. On this basis, the advantages and disadvantages of chitosan-based adsorbents were briefly analyzed.
引文
[1] R P Mason,W F Fitzgerald,F M M Morel.The biogeochemical cycling of elemental mercury:anthropogenic in?uences[J].Geochim Cosmochim Acta,1994,54:3191- 3198.
[2] 王爱勤.甲壳素化学[M].北京:科学出版社,2008:554- 563.
[3] W F Fitzgerald,D Engstrom,R P Mason,E A Nater.The case for atmospheric mercury contamination in remote areas[J].Environ Sci Technol,1998,32:1- 6.
[4] 高鹏,高彬彬,高建强,张锴,杨勇平,陈鸿伟.壳聚糖及其复合物对水中汞离子的脱除[J].化学进展,2016,12:1834- 1846.
[5] 张显,吴天星,宋小平,张云霞,汪国忠.一步溶剂热法合成磁性壳聚糖微球及其对汞离子的吸附[J].硅酸盐学报,2015,08:1143- 1149.
[6] 张娅,周颜霞,徐赛赛,陈鹏,王宏归.锰氧化物改性壳聚糖的制备及其吸附汞的研究[J].广东化工,2014,09:8- 9.
[7] S Bailey,T Olin,M Bricka,D Adrian.A review of potentially low-cost sorbents for heavy metals[J].Water Res,1999,33:2469- 2479.
[8] S Babel,T Kurniawan.Low-cost adsorbents for heavy metals uptake from contaminated water:a review[J].J Hazard Mater,2003,28:219- 243.
[9] G Crini.Recent developments in polysaccharide-based materials used adsorbents in wastewater treatment[J].Prog Polym Sci,2005,30:38- 70.
[10] A J Varma,S V Deshpande,J F Kennedy.Metal complexation by chitosan and its derivatives:a review[J].Carbohydr Polym,2004,55:77- 93.
[11] B Krajewska.Membrane-based processes performed with use of chitin/chitosan materials[J].Sep Purif Technol,2005,41:305- 312.
[12] 胡建设,张昊琳,田有粮,刘柯利.壳聚糖/硅藻土复合材料的制备及其对Hg2+吸附[J].东北大学学报,2017,09:1289- 1292.
[13] F L Mi,S S Shyu,C T Chen,J Y Lai.Adsorption of indomethacin onto chemically modi?ed chitosan beads[J].Polymer 2002,43:757- 765.
[14] 谢光勇,杜传青.壳聚糖复合材料对废水中汞离子的吸附[J].工业水处理,2009,05:24- 26.
[15] K Kurita.Chitin and chitosan:functional biopolymers from marine crustaceans [J].Mar Biotechnol,2006,8:203- 226.
[16] R Jayakumar,M Prabaharan,R L Reis,J F Mano.Graft copolymerized chitosan-present status and applications[J].Carbohydr Polym,2005,62:142- 158.
[17] 张安超,向军,孙路石,胡松,付鹏,程伟,邱建荣.新型改性吸附剂制备、表征及脱除单质汞的实验研究[J].化工学报,2009,06:1546- 1553.
[18] 张安超,孙路石,向军,高鹏,胡松,徐朝芬,付鹏.改性壳聚糖吸附剂表征及脱除Hg2+的实验研究[J].工程热物理学报,2010,09:1607- 1610.
[19] C Peniche-Covas,L W Alvarez,W Arguelles-Monal,Adsorption of mercuric ions by chitosan[J].J Appl Polym Sci,1992,46,1147- 1150.
[20] E Lopes,F dos Anjos,E Vieira,A Cestari.An alternative Avrami equation to evaluate kinetic parameters of the interaction of Hg (II) with thin chitosan membranes[J].J Colloid Interf Sci,2003,263:542- 547.
[21] E Taboada,G Cabrera,G Cardenas.Retention capacity of chitosan for copper and mercury ions[J].J Chile Chem Soc,2003,48:7- 12.
[22] E Guibal.Heterogeneous catalysis on chitosan-based materials:a review[J].Prog Polym Sci,2005,30:71- 109.
[23] A Shafaei,F Z Ashtiani,T Kaghazchi,Equilibrium studies of the sorption of Hg (II) ions onto chitosan[J].Chem Eng J,2007,133:311- 316.
[24] A Gamage,F Shahidi.Use of chitosan for the removal of metal ion contaminants and proteins from water[J].Food Chem,2007,104:989- 996.
[26] G Cardenas,O Parra,E Taboada,Synthesis and applications of chitosan mercaptanes as heavy metal retention agent[J].Int J Biol Macromol,2001,28:167- 174.
[27] Z Yang,Y Yuan,Y Wang.Synthesis and evaluation of chitosan aryl azacrownethers as adsorbents for metal ions[J].J Appl Polym Sci,2000,77:3093- 3098.
[28] L M Zhou,S R Liu,Q W Huang,Adsorption of mercury and uranyl onto poly(ethyleneimine) grafted chitosan microspheres[J].Mod Chem Ind,2007,27:175- 177,179.
[29] R Qu,C Sun C Ji,C Wang,H Chen,Y Niu,C Liang,Q Song.Preparation and metal-binding behavior of chitosan functionalized by ester and amino terminated hyperbranched polyamidoamine polymers[J].Carbohydr Res,2008,343:267- 273.
[30] M Tabakci,M Yilmaz.Synthesis of a chitosan-linked calix[4]arene chelating polymer and its sorption ability toward heavy metals and dichromate anions[J].Bioresource Technol,2008,99:6642- 6645.
[31] Y H Chang,C F Huang,W J Hsu,F C Chang.Removal of Hg2+ from aqueous solution using alginate gel containing chitosan[J].J Appl Polym Sci,2007,104:2896- 2905.
[32] B C Son,K Park,S H Song,Y J Yoo.Selective biosorption of mixed heavy metal ions using polysaccharides[J].Korean J Chem Eng,2004,21:1168- 1172.
[33] J Song,J Li,D Wang,Y Wang.Study on crosslinked carboxymethyl chitosan for adsorbing trace inorganic mercury[J].Ion Exchange Adsorption,2008,24:175- 182.
[34] A M Donia,A Atia,K Z Elwakeel.Selective separation of mercury (II) using magnetic chitosan resin modified with Schiff’s base derived from thiourea and glutaral-dehyde[J].J Hazard Mater,2008,151:372- 379.
[35] C Ni,Y Xu.Studies on syntheses and properties of chelating resins based on chitosan[J].J Appl Polym Sci,1996,59:499- 504.
[36] J D Merrifield,W G Davids,J D MacRae,A Amirbahman.Uptake of mercury by thiol-grafted chitosan gel beads[J].Water Res,2004,38:3132- 3138.
[37] N Li,R Bai,C Liu,Enhanced and selective adsorption of mercury ions on chitosan beads grafted with polyacrylamide via surface-initiated atom transfer radical polymerization,Langmuir 21 (2005) 11780- 11787.
[2] 王爱勤.甲壳素化学[M].北京:科学出版社,2008:554- 563.
[3] W F Fitzgerald,D Engstrom,R P Mason,E A Nater.The case for atmospheric mercury contamination in remote areas[J].Environ Sci Technol,1998,32:1- 6.
[4] 高鹏,高彬彬,高建强,张锴,杨勇平,陈鸿伟.壳聚糖及其复合物对水中汞离子的脱除[J].化学进展,2016,12:1834- 1846.
[5] 张显,吴天星,宋小平,张云霞,汪国忠.一步溶剂热法合成磁性壳聚糖微球及其对汞离子的吸附[J].硅酸盐学报,2015,08:1143- 1149.
[6] 张娅,周颜霞,徐赛赛,陈鹏,王宏归.锰氧化物改性壳聚糖的制备及其吸附汞的研究[J].广东化工,2014,09:8- 9.
[7] S Bailey,T Olin,M Bricka,D Adrian.A review of potentially low-cost sorbents for heavy metals[J].Water Res,1999,33:2469- 2479.
[8] S Babel,T Kurniawan.Low-cost adsorbents for heavy metals uptake from contaminated water:a review[J].J Hazard Mater,2003,28:219- 243.
[9] G Crini.Recent developments in polysaccharide-based materials used adsorbents in wastewater treatment[J].Prog Polym Sci,2005,30:38- 70.
[10] A J Varma,S V Deshpande,J F Kennedy.Metal complexation by chitosan and its derivatives:a review[J].Carbohydr Polym,2004,55:77- 93.
[11] B Krajewska.Membrane-based processes performed with use of chitin/chitosan materials[J].Sep Purif Technol,2005,41:305- 312.
[12] 胡建设,张昊琳,田有粮,刘柯利.壳聚糖/硅藻土复合材料的制备及其对Hg2+吸附[J].东北大学学报,2017,09:1289- 1292.
[13] F L Mi,S S Shyu,C T Chen,J Y Lai.Adsorption of indomethacin onto chemically modi?ed chitosan beads[J].Polymer 2002,43:757- 765.
[14] 谢光勇,杜传青.壳聚糖复合材料对废水中汞离子的吸附[J].工业水处理,2009,05:24- 26.
[15] K Kurita.Chitin and chitosan:functional biopolymers from marine crustaceans [J].Mar Biotechnol,2006,8:203- 226.
[16] R Jayakumar,M Prabaharan,R L Reis,J F Mano.Graft copolymerized chitosan-present status and applications[J].Carbohydr Polym,2005,62:142- 158.
[17] 张安超,向军,孙路石,胡松,付鹏,程伟,邱建荣.新型改性吸附剂制备、表征及脱除单质汞的实验研究[J].化工学报,2009,06:1546- 1553.
[18] 张安超,孙路石,向军,高鹏,胡松,徐朝芬,付鹏.改性壳聚糖吸附剂表征及脱除Hg2+的实验研究[J].工程热物理学报,2010,09:1607- 1610.
[19] C Peniche-Covas,L W Alvarez,W Arguelles-Monal,Adsorption of mercuric ions by chitosan[J].J Appl Polym Sci,1992,46,1147- 1150.
[20] E Lopes,F dos Anjos,E Vieira,A Cestari.An alternative Avrami equation to evaluate kinetic parameters of the interaction of Hg (II) with thin chitosan membranes[J].J Colloid Interf Sci,2003,263:542- 547.
[21] E Taboada,G Cabrera,G Cardenas.Retention capacity of chitosan for copper and mercury ions[J].J Chile Chem Soc,2003,48:7- 12.
[22] E Guibal.Heterogeneous catalysis on chitosan-based materials:a review[J].Prog Polym Sci,2005,30:71- 109.
[23] A Shafaei,F Z Ashtiani,T Kaghazchi,Equilibrium studies of the sorption of Hg (II) ions onto chitosan[J].Chem Eng J,2007,133:311- 316.
[24] A Gamage,F Shahidi.Use of chitosan for the removal of metal ion contaminants and proteins from water[J].Food Chem,2007,104:989- 996.
[26] G Cardenas,O Parra,E Taboada,Synthesis and applications of chitosan mercaptanes as heavy metal retention agent[J].Int J Biol Macromol,2001,28:167- 174.
[27] Z Yang,Y Yuan,Y Wang.Synthesis and evaluation of chitosan aryl azacrownethers as adsorbents for metal ions[J].J Appl Polym Sci,2000,77:3093- 3098.
[28] L M Zhou,S R Liu,Q W Huang,Adsorption of mercury and uranyl onto poly(ethyleneimine) grafted chitosan microspheres[J].Mod Chem Ind,2007,27:175- 177,179.
[29] R Qu,C Sun C Ji,C Wang,H Chen,Y Niu,C Liang,Q Song.Preparation and metal-binding behavior of chitosan functionalized by ester and amino terminated hyperbranched polyamidoamine polymers[J].Carbohydr Res,2008,343:267- 273.
[30] M Tabakci,M Yilmaz.Synthesis of a chitosan-linked calix[4]arene chelating polymer and its sorption ability toward heavy metals and dichromate anions[J].Bioresource Technol,2008,99:6642- 6645.
[31] Y H Chang,C F Huang,W J Hsu,F C Chang.Removal of Hg2+ from aqueous solution using alginate gel containing chitosan[J].J Appl Polym Sci,2007,104:2896- 2905.
[32] B C Son,K Park,S H Song,Y J Yoo.Selective biosorption of mixed heavy metal ions using polysaccharides[J].Korean J Chem Eng,2004,21:1168- 1172.
[33] J Song,J Li,D Wang,Y Wang.Study on crosslinked carboxymethyl chitosan for adsorbing trace inorganic mercury[J].Ion Exchange Adsorption,2008,24:175- 182.
[34] A M Donia,A Atia,K Z Elwakeel.Selective separation of mercury (II) using magnetic chitosan resin modified with Schiff’s base derived from thiourea and glutaral-dehyde[J].J Hazard Mater,2008,151:372- 379.
[35] C Ni,Y Xu.Studies on syntheses and properties of chelating resins based on chitosan[J].J Appl Polym Sci,1996,59:499- 504.
[36] J D Merrifield,W G Davids,J D MacRae,A Amirbahman.Uptake of mercury by thiol-grafted chitosan gel beads[J].Water Res,2004,38:3132- 3138.
[37] N Li,R Bai,C Liu,Enhanced and selective adsorption of mercury ions on chitosan beads grafted with polyacrylamide via surface-initiated atom transfer radical polymerization,Langmuir 21 (2005) 11780- 11787.
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