微波诱导降解有机废水的研究进展
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摘要
概括了微波的作用原理,综述了微波/吸波剂、微波/氧化剂、微波/催化剂/氧化剂联合作用在降解有机废水方面的反应条件、降解效率和原理优势,分析了微波诱导降解在处理有机废水技术中存在的问题,展望了今后的发展方向,为微波诱导降解技术的研究与应用提供参考。
The mechanism of microwave is generalized,and the reaction conditions,degradation efficiencies and action principles of microwave induction in the degradation of organic wastewater are summarized.Besides,to provide a reference for the research and industrialized application of microwave cooperated with oxidation process to the treatment of refractory organic water,the problems and the future developing directions of this technology are forecast.
The mechanism of microwave is generalized,and the reaction conditions,degradation efficiencies and action principles of microwave induction in the degradation of organic wastewater are summarized.Besides,to provide a reference for the research and industrialized application of microwave cooperated with oxidation process to the treatment of refractory organic water,the problems and the future developing directions of this technology are forecast.
引文
[1]Wang N,Zheng T,Jiang J,et al.Pilot-scale treatment of p-nitrophenol wastewater by microwave-enhanced Fenton oxidation process:Effects of system parameters and kinetics study[J].Chemical Engineering Journal,2014,239(3):351-359.
[2]Hidaka H,Saitou A,Honjou H,et al.Microwave-assisted dechlorination of polychlorobenzenes by hypophosphite anions in aqueous alkaline media in the presence of Pdloaded active carbon[J].Journal of Hazardous Materials,2007,148(1/2):22-28.
[3]Shazman A,Mizrahi S,Cogan U,et al.Examining for possible non-thermal effects during heating in a microwave oven[J].Food Chemistry,2007,103(2):444-453.
[4]Zhang Z,Shan Y,Wang J,et al.Investigation on the rapid degradation of congo red catalyzed by activated carbon powder under microwave irradiation[J].Journal of Hazardous Materials,2007,147(147):325-333.
[5]Lai T L,Yong K F,Yu J W,et al.High efficiency degradation of 4-nitrophenol by microwave-enhanced catalytic method[J].Journal of Hazardous Materials,2011,185(1):366-372.
[6]He H,Yang S,Kai Y,et al.Microwave induced catalytic degradation of crystal violet in nano-nickel dioxide suspensions[J].Journal of Hazardous Materials,2009,173(1/2/3):393-400.
[7]Ai Z,Wang Y,Xiao M,et al.Microwave-induced catalytic oxidation of Rh B by a nanocomposite of Fe@Fe2O3coreshell nanowires and carbon nanotubes[J].J Phys Chem C,2008,112(26):9847-9853.
[8]Zhang Z,Xu Y,Ma X,et al.Microwave degradation of methyl orange dye in aqueous solution in the presence of nano-TiO2-supported activated carbon(supported-TiO2/AC/MW)[J].Journal of Hazardous Materials,2012,209/210(4):271-277.
[9]王罗春,周俊,朱玲燕.微波辅助-活性炭法处理电厂EDTA锅炉清洗废水可行性研究[J].环境工程学报,2011,5(2):347-351.
[10]吴慧英,施周,陈积义,等.活性炭-微波辐射法去除苯酚的机理研究[J].环境工程学报,2009,3(1):67-71.
[11]Veksha A,Pandya P,Hill J M.The removal of methyl orange from aqueous solution by biochar and activated carbon under microwave irradiation and in the presence of hydrogen peroxide[J].Journal of Environmental Chemical Engineering,2015,3(3):1452-1458.
[12]廖建波,卜龙利,张钰彩,等.微波辐照下碳化硅与沸石负载氧化铜催化剂协同去除甲苯的实验研究[J].环境科学学报,2011,31(11):2416-2422.
[13]殷诚,周继承,尹静雅,等.微波催化剂Cu O/AC微波催化氧化降解废水中的苯酚[J].环境工程学报,2015,9(11):5329-5335.
[14]Ju Y M,Yang S G,Ding Y C,et al.Microwave-enhanced H2O2-based process for treating aqueous malachite green solutions:Intermediates and degradation mechanism[J].Journal of Hazardous Materials,2009,171(1/2/3):123-132.
[15]Zhang L,Yan F,Shu M M,et al.Investigation of the degradation behaviour of methamidophos under microwave irradiation[J].Desalination,2009,247(1/2/3):396-402.
[16]Ravera M,Buico A,Gosetti F,et al.Oxidative degradation of 1,5-naphthalenedisulfonic acid in aqueous solutions by microwave irradiation in the presence of H2O2[J].Chemosphere,2009,74(74):1309-1314.
[17]Hong J,Yuan N,Wang Y,et al.Efficient degradation of Rhodamine B in microwave-H2O2system at alkaline p H[J].Chemical Engineering Journal,2012,191(19):364-368.
[18]Lee Y C,Lo S L,Chiueh P T,et al.Efficient decomposition of perfluorocarboxylic acids in aqueous solution using microwave-induced persulfate[J].Water Research,2009,43(11):2811-2816.
[19]赵德明,张谭,张建庭,等.微波辅助二氧化氯氧化降解苯酚[J].化工学报,2011,62(7):2020-2025.
[20]Zhang L,Guo X,Yan F,et al.Study of the degradation behaviour of dimethoate under microwave irradiation[J].Journal of Hazardous Materials,2007,149(3):675-679.
[21]Zhao L,Yang S,Wang L,et al.Rapid and simple spectrophotometric determination of persulfate in water by microwave assisted decolorization of Methylene Blue[J].Journal of Environmental Sciences,2015,27(5):235-239.
[22]Bi X Y,Yang H Y,Sun P S.Microwave-induced oxidation progress for treatment of imidacloprid pesticide wastewater[J].Applied Mechanics&Materials,2012,229/230/231:2489-2492.
[23]李亚峰,高颖,王景新.微波强化Fenton/活性炭工艺处理制药废水的影响因素[J].环境工程学报,2014,8(6):2317-2321.
[24]Liu S T,Huang J,Ye Y,et al.Microwave enhanced Fenton process for the removal of methylene blue from aqueous solution[J].Chemical Engineering Journal,2013,215(2):586-590.
[25]Tan D,Zeng H,Liu J,et al.Degradation kinetics and mechanism of trace nitrobenzene by granular activated carbon enhanced microwave/hydrogen peroxide system[J].Journal of Environmental Sciences,2013,25(7):1492-1499.
[26]Yan P,Gao L B,Li W T.Microwave-enhanced Fenton-like system,Fe3O4/H2O2for Rhodamine B wastewater degradation[J].Applied Mechanics&Materials,2013,448/449/450/451/452/453:834-837.
[27]Bi X Y,Wang P,Jiang H,et al.Treatment of phenol wastewater by microwave-induced Cl O2-Cu Ox/Al2O3catalytic oxidation process[J].Journal of Environmental Sciences,2007,19(12):1510-1515.
[28]Bi X,Wang P,Jiao C,et al.Degradation of remazol golden yellow dye wastewater in microwave enhanced Cl O2catalytic oxidation process[J].Journal of Hazardous Materials,2009,168(2/3):895-900.
[29]Xie Q,Zhang Y,Chen S,et al.Generation of hydroxyl radical in aqueous solution by microwave energy using activated carbon as catalyst and its potential in removal of persistent organic substances[J].Journal of Molecular Catalysis A Chemical,2007,263(1/2):216-222.
[30]汪昆平,赵越,郭劲松,等.微波诱导AC/Cu、AC/Fe催化非均相Fenton反应催化降解垃圾渗滤液[J].环境工程学报,2012,6(11):3947-3952.
[31]占昌朝,钟明强,陈枫,等.微波诱导鳞片石墨-H2O2催化氧化处理甲基紫废水[J].环境工程学报,2013,7(11):4300-4306.
[32]丁太文,韩永忠,李茂,等.杀螟硫磷生产废水的试验研究[J].工业用水与废水,2006,37(5):34-37.
[33]张会琴,郑怀礼,廖宏头,等.微波促进类Fenton反应催化氧化降解染料吖啶橙[J].工业水处理,2010,30(8):54-57.
[34]鲁建江,李维军,陈景文,等.活性炭吸附-微波催化氧化处理番茄酱加工有机废水[J].环境科学与技术,2009,32(3):139-142.
[35]李硕,张广山,王鹏.微波-Fenton高级氧化工艺降解水中BPA[J].环境工程学报,2016,10(12):6879-6886.
[36]陈芳艳,施琦,唐玉斌.微波强化Fenton氧化法降解水中阴离子表面活性剂的研究[J].水处理技术,2011,37(6):23-26.
[37]Li P,Zhang L,Wang W,et al.Rapid catalytic microwave method to damage Microcystis aeruginosa with Fe Cl3-loaded active carbon[J].Environmental Science&Technology,2011,45(10):4521-4526.
[38]Hu Erdan,Cheng Hefa.Catalytic effect of transition metals on microwave induced degradation of atrazine in mineral micropores[J].Water Research,2014,57:8-19.
[39]Heon Lee,Young-Kwon Park,Sun-Jae Kim,et al.Rapid degradation of methyl orange using hybrid advanced oxidation process and its synergistic effect[J].Journal of Industrial and Engineering Chemistry,2016,35:205-210.
[40]Chou Y C,Lo S L,Kuo J,et al.Microwave-enhanced persulfate oxidation to treat mature landfill leachate[J].Journal of Hazardous Materials,2015,284(284):83-91.
[2]Hidaka H,Saitou A,Honjou H,et al.Microwave-assisted dechlorination of polychlorobenzenes by hypophosphite anions in aqueous alkaline media in the presence of Pdloaded active carbon[J].Journal of Hazardous Materials,2007,148(1/2):22-28.
[3]Shazman A,Mizrahi S,Cogan U,et al.Examining for possible non-thermal effects during heating in a microwave oven[J].Food Chemistry,2007,103(2):444-453.
[4]Zhang Z,Shan Y,Wang J,et al.Investigation on the rapid degradation of congo red catalyzed by activated carbon powder under microwave irradiation[J].Journal of Hazardous Materials,2007,147(147):325-333.
[5]Lai T L,Yong K F,Yu J W,et al.High efficiency degradation of 4-nitrophenol by microwave-enhanced catalytic method[J].Journal of Hazardous Materials,2011,185(1):366-372.
[6]He H,Yang S,Kai Y,et al.Microwave induced catalytic degradation of crystal violet in nano-nickel dioxide suspensions[J].Journal of Hazardous Materials,2009,173(1/2/3):393-400.
[7]Ai Z,Wang Y,Xiao M,et al.Microwave-induced catalytic oxidation of Rh B by a nanocomposite of Fe@Fe2O3coreshell nanowires and carbon nanotubes[J].J Phys Chem C,2008,112(26):9847-9853.
[8]Zhang Z,Xu Y,Ma X,et al.Microwave degradation of methyl orange dye in aqueous solution in the presence of nano-TiO2-supported activated carbon(supported-TiO2/AC/MW)[J].Journal of Hazardous Materials,2012,209/210(4):271-277.
[9]王罗春,周俊,朱玲燕.微波辅助-活性炭法处理电厂EDTA锅炉清洗废水可行性研究[J].环境工程学报,2011,5(2):347-351.
[10]吴慧英,施周,陈积义,等.活性炭-微波辐射法去除苯酚的机理研究[J].环境工程学报,2009,3(1):67-71.
[11]Veksha A,Pandya P,Hill J M.The removal of methyl orange from aqueous solution by biochar and activated carbon under microwave irradiation and in the presence of hydrogen peroxide[J].Journal of Environmental Chemical Engineering,2015,3(3):1452-1458.
[12]廖建波,卜龙利,张钰彩,等.微波辐照下碳化硅与沸石负载氧化铜催化剂协同去除甲苯的实验研究[J].环境科学学报,2011,31(11):2416-2422.
[13]殷诚,周继承,尹静雅,等.微波催化剂Cu O/AC微波催化氧化降解废水中的苯酚[J].环境工程学报,2015,9(11):5329-5335.
[14]Ju Y M,Yang S G,Ding Y C,et al.Microwave-enhanced H2O2-based process for treating aqueous malachite green solutions:Intermediates and degradation mechanism[J].Journal of Hazardous Materials,2009,171(1/2/3):123-132.
[15]Zhang L,Yan F,Shu M M,et al.Investigation of the degradation behaviour of methamidophos under microwave irradiation[J].Desalination,2009,247(1/2/3):396-402.
[16]Ravera M,Buico A,Gosetti F,et al.Oxidative degradation of 1,5-naphthalenedisulfonic acid in aqueous solutions by microwave irradiation in the presence of H2O2[J].Chemosphere,2009,74(74):1309-1314.
[17]Hong J,Yuan N,Wang Y,et al.Efficient degradation of Rhodamine B in microwave-H2O2system at alkaline p H[J].Chemical Engineering Journal,2012,191(19):364-368.
[18]Lee Y C,Lo S L,Chiueh P T,et al.Efficient decomposition of perfluorocarboxylic acids in aqueous solution using microwave-induced persulfate[J].Water Research,2009,43(11):2811-2816.
[19]赵德明,张谭,张建庭,等.微波辅助二氧化氯氧化降解苯酚[J].化工学报,2011,62(7):2020-2025.
[20]Zhang L,Guo X,Yan F,et al.Study of the degradation behaviour of dimethoate under microwave irradiation[J].Journal of Hazardous Materials,2007,149(3):675-679.
[21]Zhao L,Yang S,Wang L,et al.Rapid and simple spectrophotometric determination of persulfate in water by microwave assisted decolorization of Methylene Blue[J].Journal of Environmental Sciences,2015,27(5):235-239.
[22]Bi X Y,Yang H Y,Sun P S.Microwave-induced oxidation progress for treatment of imidacloprid pesticide wastewater[J].Applied Mechanics&Materials,2012,229/230/231:2489-2492.
[23]李亚峰,高颖,王景新.微波强化Fenton/活性炭工艺处理制药废水的影响因素[J].环境工程学报,2014,8(6):2317-2321.
[24]Liu S T,Huang J,Ye Y,et al.Microwave enhanced Fenton process for the removal of methylene blue from aqueous solution[J].Chemical Engineering Journal,2013,215(2):586-590.
[25]Tan D,Zeng H,Liu J,et al.Degradation kinetics and mechanism of trace nitrobenzene by granular activated carbon enhanced microwave/hydrogen peroxide system[J].Journal of Environmental Sciences,2013,25(7):1492-1499.
[26]Yan P,Gao L B,Li W T.Microwave-enhanced Fenton-like system,Fe3O4/H2O2for Rhodamine B wastewater degradation[J].Applied Mechanics&Materials,2013,448/449/450/451/452/453:834-837.
[27]Bi X Y,Wang P,Jiang H,et al.Treatment of phenol wastewater by microwave-induced Cl O2-Cu Ox/Al2O3catalytic oxidation process[J].Journal of Environmental Sciences,2007,19(12):1510-1515.
[28]Bi X,Wang P,Jiao C,et al.Degradation of remazol golden yellow dye wastewater in microwave enhanced Cl O2catalytic oxidation process[J].Journal of Hazardous Materials,2009,168(2/3):895-900.
[29]Xie Q,Zhang Y,Chen S,et al.Generation of hydroxyl radical in aqueous solution by microwave energy using activated carbon as catalyst and its potential in removal of persistent organic substances[J].Journal of Molecular Catalysis A Chemical,2007,263(1/2):216-222.
[30]汪昆平,赵越,郭劲松,等.微波诱导AC/Cu、AC/Fe催化非均相Fenton反应催化降解垃圾渗滤液[J].环境工程学报,2012,6(11):3947-3952.
[31]占昌朝,钟明强,陈枫,等.微波诱导鳞片石墨-H2O2催化氧化处理甲基紫废水[J].环境工程学报,2013,7(11):4300-4306.
[32]丁太文,韩永忠,李茂,等.杀螟硫磷生产废水的试验研究[J].工业用水与废水,2006,37(5):34-37.
[33]张会琴,郑怀礼,廖宏头,等.微波促进类Fenton反应催化氧化降解染料吖啶橙[J].工业水处理,2010,30(8):54-57.
[34]鲁建江,李维军,陈景文,等.活性炭吸附-微波催化氧化处理番茄酱加工有机废水[J].环境科学与技术,2009,32(3):139-142.
[35]李硕,张广山,王鹏.微波-Fenton高级氧化工艺降解水中BPA[J].环境工程学报,2016,10(12):6879-6886.
[36]陈芳艳,施琦,唐玉斌.微波强化Fenton氧化法降解水中阴离子表面活性剂的研究[J].水处理技术,2011,37(6):23-26.
[37]Li P,Zhang L,Wang W,et al.Rapid catalytic microwave method to damage Microcystis aeruginosa with Fe Cl3-loaded active carbon[J].Environmental Science&Technology,2011,45(10):4521-4526.
[38]Hu Erdan,Cheng Hefa.Catalytic effect of transition metals on microwave induced degradation of atrazine in mineral micropores[J].Water Research,2014,57:8-19.
[39]Heon Lee,Young-Kwon Park,Sun-Jae Kim,et al.Rapid degradation of methyl orange using hybrid advanced oxidation process and its synergistic effect[J].Journal of Industrial and Engineering Chemistry,2016,35:205-210.
[40]Chou Y C,Lo S L,Kuo J,et al.Microwave-enhanced persulfate oxidation to treat mature landfill leachate[J].Journal of Hazardous Materials,2015,284(284):83-91.
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