改性膨胀石墨在处理废水中的研究进展
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摘要
通过使用表面改性、金属氧化物、有机物、不同碳源等多种方法对膨胀石墨进行改性,使其吸附性能得到明显提高,同时,增强了对污水中的油类、重金属、色素和酚类等难降解物质的处理能力,对多种典型废水处理具有良好的处理效果。
Expanded graphite is modified by surface modification,metal oxide,organic matters and different carbon sources to improve its adsorption performance while to enhance its ability to treat with refractory substances in sewage such as oil,heavy metals,pigments and phenols,which has a good treatment effect on various typical wastewater.
Expanded graphite is modified by surface modification,metal oxide,organic matters and different carbon sources to improve its adsorption performance while to enhance its ability to treat with refractory substances in sewage such as oil,heavy metals,pigments and phenols,which has a good treatment effect on various typical wastewater.
引文
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[2]Toyoda M,Inagaki M. Heavy oil sorption using exfoliated graphite new application of exfoliated graphite to protect heavy oil pollution[J].Carbon,2000,38(2):199-210.
[3]Thilagavathi G,Praba Karan C,Das D. Oil sorption and retention capacities of thermally-bonded hybrid nonwovens prepared from cotton,kapok,milkweed and polypropylene fibers[J]. Journal of Environmental Management,2018,219:340-349.
[4]Toyoda M,Aizawa J,Inagaki M.Sorption and recovery of heavy oil by using exfoliated graphite[J].Spill Science&Technology Bulletin,2003,8(5):467-474.
[5]Ding X,Wang R,Zhang X,et al.A new magnetic expanded graphite for removal of oil leakage[J]. Marine Pollution Bulletin,2014,81(1):185-190.
[6]Wang X,Wang J,Zhang J,et al.Synthesis of expanded graphite C/C composites(EGC)based Ni-N-TiO2floating photocatalysts for in situ adsorption synergistic photocatalytic degradation of diesel oil[J]. Journal of Photochemistry and Photobiology A:Chemistry,2017,347:105-115.
[7]陈希.膨胀石墨基多孔炭/炭复合材料的制备及吸附性能[D].北京:清华大学,2005.
[8]Li S,Tian S,Du C,et al. Vaseline-loaded expanded graphite as a new adsorbent for toluene[J].Chemical Engineering Journal,2010,162(2):546-551.
[9]赵颖华.膨胀石墨的制备及其对金属离子去除性能的研究[D].上海:东华大学,2012.
[10]侯晓龙,刘爱琴,蔡丽平.5种物理吸附剂对模拟废水中重金属的吸附效果[J].亚热带农业研究,2012,8(2):105-112.
[11]胡珂琛,谢水波,刘迎九,等.膨胀石墨对U(Ⅵ)的吸附特性[J].环境工程学报,2016,10(3):1126-1132.
[12]焦春磊,徐从斌,李姝谚,等.羟基氧化铁/膨胀石墨复合材料的制备及除砷机制[J].高等学校化学学报,2017,38(8):1316-1323.
[13]赵颖华,李登新.改性膨胀石墨对含铅废水吸附特性[J].环境工程学报,2012,6(10):3613-3617.
[14]Jiang L,Zhang J,Xu X,et al.Characterization and application of expanded graphite modified with phosphoric acid and glucose for the removal of Ni(Ⅱ)from aqueous solution[J].Applied Surface Science,2015,357:2355-2363.
[15]Xu C,Yang W,Liu W,et al. Performance and mechanism of Cr(Ⅵ)removal by zero-valent iron loaded onto expanded graphite[J].Journal of Enviromental Sciences,2018,67(5):14-22.
[16]朱敏聪.膨胀石墨基复合材料的制备、改性及其对水中特定污染物去除的研究[D].上海:东华大学,2012.
[17]李庆,蒋丽娜,王玲,等.膨胀石墨对甲基橙废水吸附脱色的研究[J].河北农业大学学报,2009,32(1):107-109.
[18]田利强,孙根行,杨恬.膨胀石墨对活性染料的脱色性能[J].印染,2016,42(7):7-10.
[19]黎梅.超声波和膨胀石墨相结合处理染料废水的研究[D].保定:河北大学,2008.
[20]岳冬梅.超声波结合膨胀石墨及类芬顿试剂降解偶氮染料[D].石家庄:河北师范大学,2017.
[21]孙素艳.负载氧化锌膨胀石墨的制备及其对染料的脱色性能研究[D].保定:河北大学,2015.
[22]占昌朝,钟明强,陈枫,等.微波诱导改性膨胀石墨-H2O2催化氧化刚果红废水[J].环境科学与技术,2013,36(10):186-190.
[23]王会丽,赵越,马乐宽,等.复合改性膨胀石墨的制备及对酸性艳蓝染料的吸附[J].高等学校化学学报,2016,37(2):335-341.
[24]许松松,吴正颖,王赛,等.介孔SiO2/膨胀石墨复合材料的直接合成及其对染料的吸附性能[J].复合材料学报,2017,34(2):414-422.
[25]Kong Y,Yuan J,Wang Z,et al.Application of expanded graphite/attapulgite composite materials as electrode for treatment of textile wastewater[J].Applied Clay Science,2009,46(4):358-362.
[26]Kong Y,Wang Z L,Wang Y,et al.Degradation of methyl orange in artificial wastewater through electrochemical oxidation using exfoliated graphite electrode[J]. New Carbon Materials,2011,26(6):459-464.
[27]Umukoro E H,Peleyeju M G,Ngila J C,et al.Towards wastewater treatment:Photo-assisted electrochemical degradation of nitrophenol and orangeⅡdye at a tungsten trioxide-exfoliated graphite composite electrode[J]. Chemical Engineering Journal,2017,317:290-301.
[28]李冀辉.以鳞片石墨为原料的多功能碳材料的制备与应用研究[D].保定:河北大学,2009.
[29]李郑鑫.膨胀石墨的制备及其对煤炭地下气化污染地下水的净化研究[D].焦作:河南理工大学,2016.
[30]王振邦.膨胀石墨基炭炭复合材料的制备及其表面改性[D].镇江:江苏大学,2010.
[2]Toyoda M,Inagaki M. Heavy oil sorption using exfoliated graphite new application of exfoliated graphite to protect heavy oil pollution[J].Carbon,2000,38(2):199-210.
[3]Thilagavathi G,Praba Karan C,Das D. Oil sorption and retention capacities of thermally-bonded hybrid nonwovens prepared from cotton,kapok,milkweed and polypropylene fibers[J]. Journal of Environmental Management,2018,219:340-349.
[4]Toyoda M,Aizawa J,Inagaki M.Sorption and recovery of heavy oil by using exfoliated graphite[J].Spill Science&Technology Bulletin,2003,8(5):467-474.
[5]Ding X,Wang R,Zhang X,et al.A new magnetic expanded graphite for removal of oil leakage[J]. Marine Pollution Bulletin,2014,81(1):185-190.
[6]Wang X,Wang J,Zhang J,et al.Synthesis of expanded graphite C/C composites(EGC)based Ni-N-TiO2floating photocatalysts for in situ adsorption synergistic photocatalytic degradation of diesel oil[J]. Journal of Photochemistry and Photobiology A:Chemistry,2017,347:105-115.
[7]陈希.膨胀石墨基多孔炭/炭复合材料的制备及吸附性能[D].北京:清华大学,2005.
[8]Li S,Tian S,Du C,et al. Vaseline-loaded expanded graphite as a new adsorbent for toluene[J].Chemical Engineering Journal,2010,162(2):546-551.
[9]赵颖华.膨胀石墨的制备及其对金属离子去除性能的研究[D].上海:东华大学,2012.
[10]侯晓龙,刘爱琴,蔡丽平.5种物理吸附剂对模拟废水中重金属的吸附效果[J].亚热带农业研究,2012,8(2):105-112.
[11]胡珂琛,谢水波,刘迎九,等.膨胀石墨对U(Ⅵ)的吸附特性[J].环境工程学报,2016,10(3):1126-1132.
[12]焦春磊,徐从斌,李姝谚,等.羟基氧化铁/膨胀石墨复合材料的制备及除砷机制[J].高等学校化学学报,2017,38(8):1316-1323.
[13]赵颖华,李登新.改性膨胀石墨对含铅废水吸附特性[J].环境工程学报,2012,6(10):3613-3617.
[14]Jiang L,Zhang J,Xu X,et al.Characterization and application of expanded graphite modified with phosphoric acid and glucose for the removal of Ni(Ⅱ)from aqueous solution[J].Applied Surface Science,2015,357:2355-2363.
[15]Xu C,Yang W,Liu W,et al. Performance and mechanism of Cr(Ⅵ)removal by zero-valent iron loaded onto expanded graphite[J].Journal of Enviromental Sciences,2018,67(5):14-22.
[16]朱敏聪.膨胀石墨基复合材料的制备、改性及其对水中特定污染物去除的研究[D].上海:东华大学,2012.
[17]李庆,蒋丽娜,王玲,等.膨胀石墨对甲基橙废水吸附脱色的研究[J].河北农业大学学报,2009,32(1):107-109.
[18]田利强,孙根行,杨恬.膨胀石墨对活性染料的脱色性能[J].印染,2016,42(7):7-10.
[19]黎梅.超声波和膨胀石墨相结合处理染料废水的研究[D].保定:河北大学,2008.
[20]岳冬梅.超声波结合膨胀石墨及类芬顿试剂降解偶氮染料[D].石家庄:河北师范大学,2017.
[21]孙素艳.负载氧化锌膨胀石墨的制备及其对染料的脱色性能研究[D].保定:河北大学,2015.
[22]占昌朝,钟明强,陈枫,等.微波诱导改性膨胀石墨-H2O2催化氧化刚果红废水[J].环境科学与技术,2013,36(10):186-190.
[23]王会丽,赵越,马乐宽,等.复合改性膨胀石墨的制备及对酸性艳蓝染料的吸附[J].高等学校化学学报,2016,37(2):335-341.
[24]许松松,吴正颖,王赛,等.介孔SiO2/膨胀石墨复合材料的直接合成及其对染料的吸附性能[J].复合材料学报,2017,34(2):414-422.
[25]Kong Y,Yuan J,Wang Z,et al.Application of expanded graphite/attapulgite composite materials as electrode for treatment of textile wastewater[J].Applied Clay Science,2009,46(4):358-362.
[26]Kong Y,Wang Z L,Wang Y,et al.Degradation of methyl orange in artificial wastewater through electrochemical oxidation using exfoliated graphite electrode[J]. New Carbon Materials,2011,26(6):459-464.
[27]Umukoro E H,Peleyeju M G,Ngila J C,et al.Towards wastewater treatment:Photo-assisted electrochemical degradation of nitrophenol and orangeⅡdye at a tungsten trioxide-exfoliated graphite composite electrode[J]. Chemical Engineering Journal,2017,317:290-301.
[28]李冀辉.以鳞片石墨为原料的多功能碳材料的制备与应用研究[D].保定:河北大学,2009.
[29]李郑鑫.膨胀石墨的制备及其对煤炭地下气化污染地下水的净化研究[D].焦作:河南理工大学,2016.
[30]王振邦.膨胀石墨基炭炭复合材料的制备及其表面改性[D].镇江:江苏大学,2010.
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