用户名: 密码: 验证码:
电除尘器飞灰粒径表征及细颗粒降温团聚
详细信息    查看全文 | 推荐本文 |
  • 英文篇名:Fly ash particle characterization of electrostatic precipitators and cooling agglomeration for fine particles
  • 作者:刘含笑 ; 郦建国 ; 姚宇平 ; 何毓忠 ; 陈招妹 ; 王鹏
  • 英文作者:LIU Hanxiao;LI Jianguo;YAO Yuping;HE Yuzhong;CHEN Zhaomei;WANG Peng;Feida Environmental Protection Technology Co.,Ltd.;Shenhua Guohua(Beijing)Electric Power Research Institute Co.,Ltd.;
  • 关键词:低低温电除尘器 ; PM_(2.5) ; 降温团聚 ; 粒度分布 ; 除尘效率
  • 英文关键词:low-low temperature electrostatic precipitator;;PM_(2.5);;cooling agglomeration;;particle size distribution;;collection efficiency
  • 中文刊名:HGJZ
  • 英文刊名:Chemical Industry and Engineering Progress
  • 机构:浙江菲达环保科技股份有限公司;神华国华(北京)电力研究院有限公司;
  • 出版日期:2018-06-05
  • 出版单位:化工进展
  • 年:2018
  • 期:v.37;No.321
  • 基金:国家重点研发计划(2017YFB0603202)及国家重点研发计划(2016YFC0203704)
  • 语种:中文;
  • 页:HGJZ201806047
  • 页数:13
  • CN:06
  • ISSN:11-1954/TQ
  • 分类号:388-400
摘要
基于50000m~3/h实烧烟气中试系统,采用Mastersizer 2000E激光粒度分析仪和电子低压冲击仪(ELPI),首次对电除尘器飞灰几何粒径和空气动力学粒径进行全面表征。结果表明,电除尘器入口及各电场的飞灰几何粒度分布均呈双峰分布特征,各电场峰值依次右移,但末级旋转电极电场≤1μm的颗粒占比略有升高,电除尘器入口及第1~5电场飞灰几何中位径分别为6.607μm、17.378μm、2.884μm、2.577μm、2.460μm、2.480μm;温度降低,电除尘器入口飞灰几何粒度分布的双峰均右移,颗粒团聚现象明显,80℃、90℃、110℃、130℃、150℃时电除尘器入口飞灰几何中位径分别为13.183μm、10.500μm、10.171μm、6.607μm、7.586μm,从130℃降至90℃,电除尘器入口几何粒径≤1μm、≤2.5μm、≤10μm的飞灰占比分别减少了19.8%、19.2%、12.6%;不同温度时,电除尘器对空气动力学粒径0.03~10μm段颗粒的个数浓度、质量浓度均有较高脱除效率,均在75%以上,最高可达99.9%;温度降低,电除尘器进出口空气动力学粒径不同粒径段颗粒个数浓度和质量浓度均有不同程度降低,从130℃降至90℃、80℃,对应电除尘器入口PM_(2.5)团聚效率分别为46.76%、60.08%,对应电除尘器出口PM_(10)减排分别为59.80%、91.08%,PM_(2.5)减排分别为45.94%、76.22%,PM_1减排分别为40.40%、62.12%。
        Based on the 50000m~3/h actual flue gas pilot test system,the Mastersizer 2000E laser particle size analyzer and electrical low pressure impactor(ELPI)were used to fully characterize the geometric particle size and aerodynamic particle size of the fly ash particles of the electrostatic precipitator(ESP)for the first time.Results showed that,the geometric size distribution of fly ash particles of ESP inlet and different electric field is bimodal distribution characteristics,which moves to the right in turn,but particles≤1μm at the end of rotating electrode electric field have a slightly higher,the fly ash particle geometric median diameter of ESP inlet and 1—5 electric field were6.607μm,17.378μm,2.884μm,2.577μm,2.460μm,2.480μm,respectively.The fly ash particles geometric size distribution bimodal of ESP inlet moves to the right when temperature was reduced,particle agglomeration phenomenon was obvious,the fly ash particle geometric median diameter of80℃,90℃,110℃,130℃,150℃for ESP inlet were 13.183μm,10.500μm,10.171μm,6.607μm,7.586μm,from 130℃to 90℃,particles ratio of≤1μm,≤2.5μm,≤10μm decreased by 19.8%,19.8%and 19.8%respectively.At different temperatures,the ESP collection efficiency of number and mass concentration for aeordynamic diameter 0.03μm to 10μm,which were all higher than 75%,and the highest was up to 99.9%.The number and mass concentration for different period of aerodynamic diameter reduced obviously,from 130℃to 90℃and 80℃,the PM_(2.5) agglomeration efficiency of mass concentration for ESP inlet were 46.76%and 46.76%respectively.The PM_(10) reduction efficiency of mass concentration for ESP outlet were 59.80%and 91.08%.PM_(2.5) reduction efficiency were45.94%and 76.22%.PM_1 reduction efficiency were 40.40%and 62.12%,respectively.
引文
[1]中国环境保护产业协会电除尘委员会.燃煤电厂烟气超低排放技术[M].北京:中国电力出版社,2015:12-24.China Association of Environmental Protection Industry.Technology of flue gas ultra-low emission for coal-fired power plant[M].Beijing:China Electric Power Press,2015:12-24.
    [2]中国环境保护产业协会.电除尘器选型设计指导书[M].北京:中国电力出版社,2013:62-64.China Association of Environmental Protection Industry.ESP design instruction[M].Beijing:China Electric Power Press,2013:62-64.
    [3]闫克平,李树然,冯卫强,等.高电压环境工程应用研究关键技术问题分析及展望[J].高电压技术,2015,41(8):2528-2544.YAN Keping,LI Shuran,FENG Weiqiang,et al.Development and application of electrostatic precipitation technology[J].High Voltage Engineering,2015,41(8):2528-2544.
    [4]郦建国,刘云.中国煤种成分对电除尘器性能影响及电除尘器适应性评价[J].科技导报,2010,28(7):104-109.LI Jianguo,LIU Yun.The effect of compositions of domestic coal on the performance of ESP and an evaluation of ESP adaptability[J].Science&Technology Review,2010,28(7):104-109.
    [5]刘忠,刘含笑,冯新新,等.湍流聚并器流场和颗粒运动轨迹模拟[J].中国电机工程学报,2012,32(14):71-75.LIU Zhong,LIU Hanxiao,FENG Xinxin,et al.Simulation for the flow field of the turbulence coalescence device and the trajectory of particles[J].Proceedings of the CSEE,2012,32(14):71-75.
    [6]章鹏飞,米建春,潘祖明.烟气流速和装置元件角度对细颗粒湍流聚并的影响[J].中国电机工程学报,2016,36(10):2714-2720.ZHANG Pengfei,MI Jianchun,PAN Zuming.Influences of flue-gas velocity and device-element angle on fine particle amalgamation[J].Proceedings of the CSEE,2016,36(10):2714-2720.
    [7]MORI Yusuke,TSUMITA Yoshimitsu,MATSUMOTO Ario,et al.Operation results of IHI flue gas desulfurization system-unit No.1(1000MW)of hitachinaka thermal power station for TEPCO[J].IHI Engineering Review,2006,39(1):22-26.
    [8]MASAMI Kato,TADASHI Tanaka,YASUKI Nishimura,et al.Method and system for handling exhaust gas in a boiler:US5282429[P].1994-02-01.
    [9]YOSHIO Nakayama,SATOSHI Nakamura,YASUHIRO Takeuchi,et al.MHI high efficiency system-Proven technology for multi pollutant removal[R].Hiroshima Research&Development Center.2011:1-11.
    [10]名嶋慎司.石炭火力用低低温電気集塵装置[J].住友重機械技報,2001,146:35-38.
    [11]郦建国,郦祝海,何毓忠,等.低低温电除尘技术的研究及应用,中国环保产业,2014(3):28-34.LI Jianguo,LI Zhuhai,HE Yuzhong,et al.Research and application on electric precipitation technology with low-low temperature[J].China Environmental Protection Industry,2014(3):28-34.
    [12]郦建国,郦祝海,李卫东,等.燃煤电厂烟气协同治理技术路线研究[J].中国环保产业,2015(5):52-56.LI Jianguo,LI Zhuhai,LI Weidong,et al.Research on flue gas co-benefit control technical route in coal-fired power plants[J].China Environmental Protection Industry,2015(5):52-56.
    [13]何毓忠,何海涛,胡露钧,等.低低温电除尘技术的工程应用[J].中国环保产业,2016(4):22-24HE Yuzhong,HE Haitao,HU Lujun,et al.Engineering application of electric precipitation technology with low-low temperature[J].China Environmental Protection Industry,2016(4):22-24.
    [14]刘含笑,姚宇平,郦建国,等.燃煤电厂烟气中SO3生成、治理及测试技术研究[J].中国电力,2015,48(9):152-156.LIU Hanxiao,YAO Yuping,LI Jianguo,et al.Study on SO3generation,control and testing technology for coal-fired power plants[J].Electric Power,2015,48(9):152-156.
    [15]刘含笑,袁建国,郦祝海,等.低低温工况下颗粒凝并机理分析及研究方法初探[J].电力与能源,2015,36(1):107-111.LIU Hanxiao,YUAN Jianguo,LI Zhuhai,et al.Tentative study on mechanism analysis and research method of particle coagulation in low-low temperature working condition[J].Power of Energy,2015,36(1):107-111.
    [16]王树民,张翼,刘吉臻.燃煤电厂细颗粒物控制技术集成应用及“近零排放”特性[J].环境科学研究,2016,29(9):1256-1263.WANG Shumin,ZHANG Yi,LIU Jizhen.Integrated application of fine particulate matter control technologies and their“near-zero emission”characteristics in coal-fired power plants[J].Research of Environmental Sciences,2016,29(9):1256-1263.
    [17]寿春晖,祁志福,谢尉扬,等.低低温电除尘器颗粒物脱除特性的工程应用试验研究[J].中国电机工程学报,2016,36(16):4326-4332.SHOU Chunhui,QI Zhifu,XIE Weiyang,et al.Experimental study on engineering application of particulate matter removal characteristics of low-low temperature electrostatic precipitator[J].Proceedings of the CSEE,2016,36(16):4326-4332.
    [18]莫华,朱法华,王圣.火电行业大气污染物排放对PM2.5的贡献及减排对策[J].中国电力,2013,46(8):1-6.MO Hua,ZHU Fahua,WANG Sheng.Contribution to PM2.5 of atmospheric pollutant emission from thermal power sector and emission reduction countermeasures[J].Electric Power,2013,46(8):1-6.
    [19]刘含笑,姚宇平,郦建国,等.PM2.5团聚测试技术及其研究进展[J].电力与能源,2013(4):118-123.LIU Hanxiao,YAO Yuping,LI Jianguo,et el.The measurement technology and research progress of the PM2.5 coalescence experiment[J].Power&Energy,2013(4):118-123.
    [20]朱少平,刘含笑,郦建国,等.电子低压冲击器不同稀释比对PM2.5排放测试的影响[J].电力与能源,2014(2):141-143.ZHU Shaoping,LIU Hanxiao,LI Jianguo,et al.The influence of PM2.5 emission test with the method of ELPI different dilution ratio[J].Power&Energy,2014(2):141-143.
    [21]刘含笑,朱少平,姚宇平,等.电荷法测试WESP进出口烟气中PM2.5的试验研究[J].中国电力,2014,47(12):37-41.LIU Hanxiao,ZHU Shaoping,YAO Yuping,et al.Inlet and outlet flue gas PM2.5 test experimental research with ELPI for WESP of“ultra-clean emission”power plant[J].Electric Power,2014,47(12):37-41.
    [22]HUANG S H,CHEN C C.Ultrafine aerosol penetration through electrostatic precipitators[J].Aerosol Science and Technology,2002,36(21):4625-4632.
    [23]ZHU Jibao,ZHAO Qinxia,YAO Yuping,et al.Effects of high-voltage power sources on fine particle collection efficiency with an industrial electrostatic precipitator[J].Journal of Electrostatics,2012,70(7):285-291.
    [24]HUANG S H,CHEN C C.Filtration characteristics of a miniature electrostatic precipitator[J].Aerosol Science and Technology,2001,35(4):792-804.
    [25]MISAK T,AKASAKA A,YABUTA H.Recent applications of moving electrode type electrostatic precipitator[C]//International Society for Electrostatic Precipitation.Proceedings of the 7th International Conference on Electrostatic Precipitation,Korean,1998:508-515.
    [26]MISAKA T,OURA T,YAMAZAKI M.Improvement of reliability for moving electrode type electrostatic precipitator[C]//International Society for Electrostatic Precipitation.Proceedings of the 10th International Conference on Electrostatic Precipitation,Australia,2006:1-4
    [27]王仕龙,陈英,韩平,等.燃煤电厂电除尘PM10和PM2.5的排放控制Ⅰ:电除尘选型及工业应用[J].科技导报,2014,32(33):23-33.WANG Shilong,CHEN Ying,HAN Ping,et al.PM10 and PM2.5emission control by electrostatic precipitator(ESP)for coal-fired power plants I:ESP sizing and applications[J].Science&Technology Review,2014,32(33):23-33.
    [28]USH P V.Study of rapping reentrainment emissions from a pilot-scale electrostatic precipitator[J].Environmental Science&Technology,1984,18(9):699-705.
    [29]ENGELBRECHT H L.Rapping systems for collecting surfaces in an electrostatic precipitator[J].Environment International,1981,6(1/6):297-305.
    [30]李志敏.燃煤锅炉排烟的酸-灰耦合作用与露点的动态变化机制研究[D].济南:山东大学,2016.LI Zhimin.Research on acid-grey coupling mechanism and dew point dynamic charateristics of coal-fired boiler flue gas[D].Jinan:Shangdong University,2016.
    [31]中华人民共和国环境保护部.火电厂污染防治可行技术指南:HJ 2301—2017[S].北京:中国标准出版社,2017.Ministry of Environmental Protection of the People's Republic of China.Guideline on best available technologies of pollution prevention and control for thermal power plant:HJ 2301—2017[S].Beijing:Standards Press of China,2017.
    [32]熊桂龙,李水清,陈晟,等.增强PM2.5脱除的新型电除尘技术的发展[J].中国电机工程学报,2015,35(9):2217-2223.XIONG Guilong,LI Shuiqing,CHEN Sheng,et al.Development of adcanced electrostatic precipitation technologies for reducing PM2.5emissions from coal-fired power plants[J].Proceedings of the CSEE,2015,35(9):2217-2223.
    [33]魏凤,张军营,王春梅,等.煤燃烧超细颗粒物团聚促进技术的研究进展[J].煤炭转化,2003,26(3):27-31.WEI Feng,ZHANG Junying,WANG Chunmei,et al.Review of submicron particles agglomeration in coal combustion process[J].Coal Conversion,2003,26(3):27-31.
    [34]刘忠,刘含笑,冯新新,等.超细颗粒物聚并模型的比较研究[J].燃烧科学与技术,2012,18(3):212-216.LIU Zhong,LIU Hanxiao,FENG Xinxin,et al.Comparative study on the different coalescence models of ultrafine particles[J].Journal of Combustion Science and Technology,2012,18(3):212-216.
    [35]刘含笑,姚宇平,郦建国.凝聚器二维单扰流柱流场中颗粒凝并模拟[J].动力工程学报,2015,35(4):292-297.LIU Hanxiao,YAO Yuping,LI Jianguo.Coagulating simulation of particles in flow field of coagulator 2D single turbulence column[J].Journal of Chinese Society of Power Engineering,2015,35(4):292-297.
    [36]李林,董勇,崔琳,等.荷电水雾脱除超细颗粒物的研究进展[J].化工进展,2010,29(6):1143-1147.LI Lin,DONG Yong,CUI Lin,et al.Removal of submicron particles by charged water droplets[J].Chemical Industry and Engineering Progress,2010,29(6):1143-1147.
    [37]刘勇,赵汶,刘瑞,等.化学团聚促进电除尘脱除PM2.5的实验研究[J].化工学报,2014,65(9):3609-3616.LIU Yong,ZHAO Wen,LIU Rui,et al.Improving removal of PM2.5by electrostatic precipitator with chemical agglomeration[J].CIESC Journal,2014,65(9):3609-3616.
    [38]胡斌,刘勇,杨春敏,等.化学团聚促进电除尘脱除烟气中PM2.5和SO3[J].化工学报,2016,67(9):3902-3909.HU Bin,LIU Yong,YANG Chunmin,et al.Simultaneous control of PM2.5 and SO3 by chemical agglomeration collaborative electrostatic precipitation[J].CIESC Journal,2016,67(9):3902-3909.
    [39]赵永椿,张军营,魏凤,等.燃煤超细颗粒物团聚促进机制的实验研究[J].化工学报,2007,58(11):2876-2881.ZHAO Yongchun,ZHANG Junying,WEI Feng,et al.Experimental study on agglomeration of submicron particles from coal combustion[J].CIESC Journal,2007,58(11):2876-2881.
    [40]张绪辉.低低温电除尘器对细颗粒物及三氧化硫的协同脱除研究[D].北京:清华大学,2015:51-53.ZHANG Xuhui.Studies on synergetic removal of fine particulates and SO3 by an extra cold-side electrostatic precipitator[D].Beijing:Tsinghua University,2015:51-53.
    [41]史文峥,杨萌萌,张绪辉,等.燃煤电厂超低排放技术路线与协同脱除[J].中国电机工程学报,2016,36(16):4308-4318.SHI Wenzheng,YANG Mengmeng,ZHANG Xuhui,et al.Ultra-low emission technical route of coal-fired power plants and the cooperative removal[J].Proceedings of the CSEE,2016,36(16):4308-4318.

© 2004-2018 中国地质图书馆版权所有 京ICP备05064691号 京公网安备11010802017129号

地址:北京市海淀区学院路29号 邮编:100083

电话:办公室:(+86 10)66554848;文献借阅、咨询服务、科技查新:66554700