高温自蔓延反应合成功能材料的研究进展
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摘要
简要总结了自蔓延高温反应(SHS)的国内外发展过程。从SHS前驱体元素体系的组成及SHS产物的应用方向(粉体功能材料、陶瓷材料、涂层材料等)进行了分类阐述,着重分析了未来含能材料在SHS方面的应用。其次,重点分析了适用于不同应用方向SHS材料的点火机制、反应机制、热力学和动力学等理论分析,在此基础上提出绝热温度不是SHS反应唯一判据的新观点。最后,介绍了自蔓延高温反应的燃烧机理,阐明了反应物粒径、球磨参数、反应物压坯压力等工艺参数对SHS反应的影响,同时对SHS技术发展中存在问题进行了分析。
The development process of self-propagating high-temperature synthesis(SHS)at home and abroad was briefly summarized.The components of the element system of SHS precursor and the application direction of SHS products(powdered functional materials,ceramic materials,coating materials)were classified and expounded and the application of future energetic materials in SHS was emphatically analyzed.Secondly,the theoretical analysis of ignition mechanism,reaction mechanism,thermodynamics and kinetics of SHS materials suitable for different application directions was emphatically analyzed.On this basis,a new viewpoint that the adiabatic temperature was not the only criterion of SHS reaction was proposed.Finally,the combustion mechanism of SHS was introduced and the effects of experimental conditions such as particle sizes of reactants,milling parameters and pressed compact pressure of reactants on the SHS reactions were clarified.At the same time,the problems in the development of the SHS technology were analyzed.
The development process of self-propagating high-temperature synthesis(SHS)at home and abroad was briefly summarized.The components of the element system of SHS precursor and the application direction of SHS products(powdered functional materials,ceramic materials,coating materials)were classified and expounded and the application of future energetic materials in SHS was emphatically analyzed.Secondly,the theoretical analysis of ignition mechanism,reaction mechanism,thermodynamics and kinetics of SHS materials suitable for different application directions was emphatically analyzed.On this basis,a new viewpoint that the adiabatic temperature was not the only criterion of SHS reaction was proposed.Finally,the combustion mechanism of SHS was introduced and the effects of experimental conditions such as particle sizes of reactants,milling parameters and pressed compact pressure of reactants on the SHS reactions were clarified.At the same time,the problems in the development of the SHS technology were analyzed.
引文
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[15]Yi H C,Varma A,A S R,et al.Gravity-Induced Microstructural Nonuniformities during Combustion Synthesis of IntermetallicCeramic Composite Materials[J].Industrial&Engineering Chemistry Research,2014,35(9):2982-2985.
[16]Sina H,Iyengar S.Studies on the formation of aluminides in heated Nb-Al powder mixtures[J].Journal of Alloys&Compounds,2014(628):9-19.
[17]Sundaram D S,Puri P,Yang V.Thermochemical Behavior of Nickel-Coated Nanoaluminum Particles[J].Journal of Physical Chemistry C,2013,117(15):7858-7869.
[18]Vallauri D,Shcherbakov V A,Khitev A V,et al.Study of structure formation in TiC-TiB2-MexOy,ceramics fabricated by SHS and densification[J].Acta Materialia,2008,56(6):1380-1389.
[19]Amosov A P,Bichurov G V,Kondrat′Eva L A,et al.Nitride nanopowders by azide SHS technology[J].International Journal of SelfPropagating High-Temperature Synthesis,2017,26(1):11-21.
[20]Mishra S K,Das S K,Sherbacov V.Fabrication of Al2O3-ZrB2,in situ composite by SHS dynamic compaction:A novel approach[J].Composites Science&Technology,2007,67(11-12):2447-2453.
[21]Baras F,Mukasyan A S,et al.Microstructure development during NiAl intermetallic synthesis in reactive Ni-Al nanolayers:Numerical investigations vs.TEM observations[J].Surface&Coatings Technology,2013,215(215):485-492.
[22]Nersisyan H H,Lee J H,Won C W.Self-propagating high-temperature synthesis of nano-sized titanium carbide powder[J].Journal of Materials Research,2002,17(11):2859-2864..
[23]Sharifi H,Hassanzadeh-Tabrizi S A,Davoodi D,et al.Investigation on mechanochemical combustion behavior of Mg-V2O5-Co3O4-C reactive system to synthesize VC-Co nanocomposite powder[J].Ceramics International,2016,42(6):7210-7215.
[24]Hassanzadeh-Tabrizi S A,Davoodi D,Beykzadeh A A,et al.Fast synthesis of VC and V2C nanopowders by the mechanochemical combustion method[J].International Journal of Refractory Metals&Hard Materials,2015(51):1-5.
[25]Pampuch R,Stobierski L,Lis J.Synthesis of Sinterable-SiC Powders by a Solid Combustion Method[J].Cheminform,1989,72(8):1434-1435.
[26]Moskovskikh D O,Lin Y C,Rogachev A S,et al.Spark plasma sintering of SiC powders produced by different combustion synthesis routes[J].Journal of the European Ceramic Society,2015,35(2):477-486.
[27]Liang Y,Han Z,Zhang Z,et al.Effect of Cu content in Cu-Ti-B4C system on fabricating TiC/TiB2,particulates locally reinforced steel matrix composites[J].Materials&Design,2012(40):64-69.
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