难降解有机废水厌氧生物处理技术现状及发展
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摘要
厌氧生物处理技术由于经济性和高效性广泛应用于难降解有机废水的治理。基于对传统厌氧生物处理技术的原理及技术现状的分析,总结了零价铁耦合厌氧生物处理难降解有机废水的原理及近些年的发展,展望了厌氧生物处理技术的未来发展趋势。
Anaerobic biological technology is widely used for treatment of hard degradable organic wastewater due to its economical efficiency and high efficiency.Based on the analysis of the principle and current status of traditional anaerobic biological treatment technology,the principle and recent developments of hard degradable organic wastewater treatment by anaerobic biological technology coupled with zero-valent iron were summarized,and finally,the feature development trend of anaerobic biological technology was forecasted.
Anaerobic biological technology is widely used for treatment of hard degradable organic wastewater due to its economical efficiency and high efficiency.Based on the analysis of the principle and current status of traditional anaerobic biological treatment technology,the principle and recent developments of hard degradable organic wastewater treatment by anaerobic biological technology coupled with zero-valent iron were summarized,and finally,the feature development trend of anaerobic biological technology was forecasted.
引文
[1]REN J,LI J,CHEN Z,et al.Fate and wetting potential of biorefractory organics in membrane distillation for coke wastewater treatment[J].Chemosphere,2018,208:450-459.
[2]ZHANG D,LI W,HOU C,et al.Aerobic granulation accelerated by biochar for the treatment of refractory wastewater[J].Chem Eng J,2017,314:88-97.
[3]YANG J,ZHANG L,XU K,et al.Using combined multiple techniques to characterize refractory organics during anammox process with mature coal chemical wastewater as influent[J].Environ Sci Pollut R,2018,25(9):1-12.
[4]ZHANG M,WANG Z,LI P,et al.Bio-refractory dissolved organic matter and colorants in cassava distillery wastewater:Characterization,coagulation treatment and mechanisms[J].Chemosphere,2017,178:259-267.
[5]张海燕,刘文聪,姜辉,等.Fenton-混凝沉淀-水解酸化-A/O工艺处理医药废水[J].中国给水排水,2018,34(4):89-92.
[6]衷从强,梁林玥,韩卫清,等.电催化氧化处理三唑类杀菌剂模拟废水[J].环境工程学报,2016,10(2):755-760.
[7]曾旭,刘俊,赵建夫.湿式氧化法预处理高浓度合成制药废水的研究[J].工业水处理,2017,37(8):78-80.
[8]SUN F,SUN B,HU J,et al.Organics and nitrogen removal from textile auxiliaries wastewater with A2O-MBR in a pilot-scale[J].JHazard Mater,2015,286:416-424.
[9]WU L N,LIANG D W,XU Y Y,et al.A robust and costeffective integrated process for nitrogen and bio-refractory organics removal from landfill leachate via short-cut nitrification,anaerobic ammonium oxidation in tandem with electrochemical oxidation[J].Bioresour Technol,2016,212:296-301.
[10]CHEN R,NIE Y,KATO H,et al.Methanogenic degradation of toilet-paper cellulose upon sewage treatment in an anaerobic membrane bioreactor at room temperature[J].Bioresour Technol,2017,228:69-76.
[11]APPELS L,BAEYENS J,DEGR魬VE J,et al.Principles and potential of the anaerobic digestion of waste-activated sludge[J].Prog Energy Combust Sci,2008,34(6):755-781.
[12]王凯军.低浓度污水厌氧-水解处理工艺[M].北京:中国环境科学出版社,1991.
[13]李绍衡.厌氧生物处理技术的原理及其在城市污水处理中的应用[J].湖南大学学报:自然科学版,2001,(S1):20-26.
[14]BRYANT M P.Microbial methane production:theoretical aspects[J].J Anim Sci,1979,48(1):193-201.
[15]ZEIKUS J G.Microbial populations in digesters[C].London:Applied Science Publishers,1980.
[16]GUJER W.Conversion processes in anaerobic digestion[J].Water Sci Technol,1983,15:127-167.
[17]贺延龄.废水的厌氧生物处理[M].北京:中国轻工业出版社,1998.
[18]LETTINGA G,VAN VELSEN A F M,HOBMA S W,et al.Use of the upflow sludge blanket(USB)reactor concept for biological wastewater treatment,especially for anaerobic treatment[J].Biotechnol Bioeng,1980,22(4):699-734.
[19]BACHMANN A,BEARD V L,MCCARTY P L.Comparison of fixed-film reactors with a modified sludge blanket reactor[R].Stanford Univ Calif Dept of Civil Engineering,1982.
[20]BARBER W P,STUCKEY D C.The use of the anaerobic baffled reactor(ABR)for wastewater treatment:a review[J].Water Res,1999,33(7):1559-1578.
[21]杨梓亨,宋卫锋,程亚杰,等.ABR反应器处理苯胺黑药废水及其微生物种群结构[J].环境科学研究,2017,30(9):1448-1454.
[22]LETTINGA G,FIELD J,LIER J V,et al.Advanced anaerobic wastewater treatment in the near future[J].Water Sci Technol,1996,35(10):5-12.
[23]SCHERER M M,JOHNSON K M,WESTALL J C,et al.Mass transport effects on the kinetics of nitrobenzene reduction by iron metal[J].Environ Sci Technol,2001,35(13):2804-2811.
[24]NOUBACTEP.Metallic iron for water treatment:a critical review[J].Acta Hydroch Hydrob,2013,41(7):702-710.
[25]刘继伟,袁合涛,杜玉凤,等.零价铁颗粒吸附材料的制备及其性能研究[J].工业用水与废水,2018,49(6):50-56.
[26]李杰,张艳梅,马宁.复合零价铁生物填料的优化试验研究[J].工业用水与废水,2015,46(4):20-22.
[27]LIANG L,GUAN X,SHI Z,et al.Coupled effects of aging and weak magnetic fields on sequestration of selenite by zero-valent iron[J].Environ Sci Technol,2014,48(11):6326-6334.
[28]YAN W,RAMOS M A V,KOEL B E,et al.As(III)sequestration by iron nanoparticles:study of solid-phase redox transformations with X-ray photoelectron spectroscopy[J].J Phys Chem,2017,116(9):5303-5311.
[29]ALVAREZ P J,TILL B A,WEATHERS L J,et al.Fe(o)-based bioremediation of aquifers contaminated with mixed wastes:US 6719902[P].2004-04-13.
[30]XIN Y,YONG K,DUUJONG L,et al.Bioaugmented sulfate reduction using enriched anaerobic microflora in the presence of zero valent iron[J].Chemosphere,2008,73(9):1436-1441.
[31]ZHANG J,ZHANG Y,XIE Q,et al.Bioaugmentation and functional partitioning in a zero valent iron-anaerobic reactor for sulfate-containing wastewater treatment[J].Chem Eng J,2011,174(1):159-165.
[32]ZHANG Y,JING Y,QUAN X,et al.A built-in zero valent iron anaerobic reactor to enhance treatment of azo dye wastewater[J].Water Sci Technol,2011,63(4):741-746.
[33]KIM Y H,CARRAWAY E R.Dechlorination of pentachlorophenol by zero valent iron and modified zero valent irons[J].Environ Sci Technol,2000,34(10):2014-2017.
[34]YI Z J,LIAN B,YANG Y Q,et al.Treatment of simulated wastewater from in situ leaching uranium mining by zerovalent iron and sulfate reducing bacteria[J].Trans Nonferrous Met Soc China,2009,19(3):s840-s844.
[35]LIU Y,ZHANG Y,QUAN X,et al.Applying an electric field in a built-in zero valent iron---anaerobic reactor for enhancement of sludge granulation[J].Water Res,2011,45(3):1258-1266.
[36]XU X,LIN H,ZHU L,et al.Enhanced biodegradation of 2-chloronitro-benzene using a coupled zero-valent iron column and sequencing batch reactor system[J].J Chem Technol Biotechnol,2011,86(7):993-1000.
[37]ZHANG J,ZHANG Y,YANG L,et al.Enhancement of nitrogen removal in a novel anammox reactor packed with Fe electrode[J].Bioresour Technol,2012,114(3):102-108.
[38]KARRI S,SIERRAALVAREZ R,FIELD J A.Zero valent iron as an electron-donor for methanogenesis and sulfate reduction in anaerobic sludge[J].Biotechnol Bioeng,2005,92(7):810-819.
[39]马斌,张耀斌,全燮,等.ZVI强化厌氧处理高浓度颜料废水[J].环境工程学报,2015,9(2):767-772.
[40]徐浩,韩洪军,魏江波,等.零价铁强化上流式厌氧污泥床反应器处理煤化工费托合成废水研究[J].环境污染与防治,2017,39(8):845-850.
[41]刘轶文.零价铁强化厌氧废水处理的研究[D].大连:大连理工大学,2011.
[42]THRASH J C,COATES J D.Review:direct and indirect electrical stimulation of microbial metabolism[J].Environ Sci Technol,2008,42(11):3921-3931.
[43]SASAKI K,SASAKI D,MORITA M,et al.Bioelectrochemical system stabilizes methane fermentation from garbage slurry[J].Bioresour Technol,2010,101(10):3415-3422.
[44]NING X A,WEN W,ZHANG Y,et al.Enhanced dewaterability of textile dyeing sludge using micro-electrolysis pretreatment[J].J Environ Manage,2015,161:181-187.
[45]XIAO X,SHENG G P,MU Y,et al.A modeling approach to describe zvi-based anaerobic system[J].Water Res,2013,47(16):6007.
[46]OU C,SHEN J,ZHANG S,et al.Coupling of iron shavings into the anaerobic system for enhanced 2,4-dinitroanisole reduction in wastewater[J].Water Res,2016,101:457-466.
[47]WU D,ZHEN S,DING A,et al.Performance of a zero valent iron-based anaerobic system in swine wastewater treatment[J].JHazard Mater,2015,286:1-6.
[2]ZHANG D,LI W,HOU C,et al.Aerobic granulation accelerated by biochar for the treatment of refractory wastewater[J].Chem Eng J,2017,314:88-97.
[3]YANG J,ZHANG L,XU K,et al.Using combined multiple techniques to characterize refractory organics during anammox process with mature coal chemical wastewater as influent[J].Environ Sci Pollut R,2018,25(9):1-12.
[4]ZHANG M,WANG Z,LI P,et al.Bio-refractory dissolved organic matter and colorants in cassava distillery wastewater:Characterization,coagulation treatment and mechanisms[J].Chemosphere,2017,178:259-267.
[5]张海燕,刘文聪,姜辉,等.Fenton-混凝沉淀-水解酸化-A/O工艺处理医药废水[J].中国给水排水,2018,34(4):89-92.
[6]衷从强,梁林玥,韩卫清,等.电催化氧化处理三唑类杀菌剂模拟废水[J].环境工程学报,2016,10(2):755-760.
[7]曾旭,刘俊,赵建夫.湿式氧化法预处理高浓度合成制药废水的研究[J].工业水处理,2017,37(8):78-80.
[8]SUN F,SUN B,HU J,et al.Organics and nitrogen removal from textile auxiliaries wastewater with A2O-MBR in a pilot-scale[J].JHazard Mater,2015,286:416-424.
[9]WU L N,LIANG D W,XU Y Y,et al.A robust and costeffective integrated process for nitrogen and bio-refractory organics removal from landfill leachate via short-cut nitrification,anaerobic ammonium oxidation in tandem with electrochemical oxidation[J].Bioresour Technol,2016,212:296-301.
[10]CHEN R,NIE Y,KATO H,et al.Methanogenic degradation of toilet-paper cellulose upon sewage treatment in an anaerobic membrane bioreactor at room temperature[J].Bioresour Technol,2017,228:69-76.
[11]APPELS L,BAEYENS J,DEGR魬VE J,et al.Principles and potential of the anaerobic digestion of waste-activated sludge[J].Prog Energy Combust Sci,2008,34(6):755-781.
[12]王凯军.低浓度污水厌氧-水解处理工艺[M].北京:中国环境科学出版社,1991.
[13]李绍衡.厌氧生物处理技术的原理及其在城市污水处理中的应用[J].湖南大学学报:自然科学版,2001,(S1):20-26.
[14]BRYANT M P.Microbial methane production:theoretical aspects[J].J Anim Sci,1979,48(1):193-201.
[15]ZEIKUS J G.Microbial populations in digesters[C].London:Applied Science Publishers,1980.
[16]GUJER W.Conversion processes in anaerobic digestion[J].Water Sci Technol,1983,15:127-167.
[17]贺延龄.废水的厌氧生物处理[M].北京:中国轻工业出版社,1998.
[18]LETTINGA G,VAN VELSEN A F M,HOBMA S W,et al.Use of the upflow sludge blanket(USB)reactor concept for biological wastewater treatment,especially for anaerobic treatment[J].Biotechnol Bioeng,1980,22(4):699-734.
[19]BACHMANN A,BEARD V L,MCCARTY P L.Comparison of fixed-film reactors with a modified sludge blanket reactor[R].Stanford Univ Calif Dept of Civil Engineering,1982.
[20]BARBER W P,STUCKEY D C.The use of the anaerobic baffled reactor(ABR)for wastewater treatment:a review[J].Water Res,1999,33(7):1559-1578.
[21]杨梓亨,宋卫锋,程亚杰,等.ABR反应器处理苯胺黑药废水及其微生物种群结构[J].环境科学研究,2017,30(9):1448-1454.
[22]LETTINGA G,FIELD J,LIER J V,et al.Advanced anaerobic wastewater treatment in the near future[J].Water Sci Technol,1996,35(10):5-12.
[23]SCHERER M M,JOHNSON K M,WESTALL J C,et al.Mass transport effects on the kinetics of nitrobenzene reduction by iron metal[J].Environ Sci Technol,2001,35(13):2804-2811.
[24]NOUBACTEP.Metallic iron for water treatment:a critical review[J].Acta Hydroch Hydrob,2013,41(7):702-710.
[25]刘继伟,袁合涛,杜玉凤,等.零价铁颗粒吸附材料的制备及其性能研究[J].工业用水与废水,2018,49(6):50-56.
[26]李杰,张艳梅,马宁.复合零价铁生物填料的优化试验研究[J].工业用水与废水,2015,46(4):20-22.
[27]LIANG L,GUAN X,SHI Z,et al.Coupled effects of aging and weak magnetic fields on sequestration of selenite by zero-valent iron[J].Environ Sci Technol,2014,48(11):6326-6334.
[28]YAN W,RAMOS M A V,KOEL B E,et al.As(III)sequestration by iron nanoparticles:study of solid-phase redox transformations with X-ray photoelectron spectroscopy[J].J Phys Chem,2017,116(9):5303-5311.
[29]ALVAREZ P J,TILL B A,WEATHERS L J,et al.Fe(o)-based bioremediation of aquifers contaminated with mixed wastes:US 6719902[P].2004-04-13.
[30]XIN Y,YONG K,DUUJONG L,et al.Bioaugmented sulfate reduction using enriched anaerobic microflora in the presence of zero valent iron[J].Chemosphere,2008,73(9):1436-1441.
[31]ZHANG J,ZHANG Y,XIE Q,et al.Bioaugmentation and functional partitioning in a zero valent iron-anaerobic reactor for sulfate-containing wastewater treatment[J].Chem Eng J,2011,174(1):159-165.
[32]ZHANG Y,JING Y,QUAN X,et al.A built-in zero valent iron anaerobic reactor to enhance treatment of azo dye wastewater[J].Water Sci Technol,2011,63(4):741-746.
[33]KIM Y H,CARRAWAY E R.Dechlorination of pentachlorophenol by zero valent iron and modified zero valent irons[J].Environ Sci Technol,2000,34(10):2014-2017.
[34]YI Z J,LIAN B,YANG Y Q,et al.Treatment of simulated wastewater from in situ leaching uranium mining by zerovalent iron and sulfate reducing bacteria[J].Trans Nonferrous Met Soc China,2009,19(3):s840-s844.
[35]LIU Y,ZHANG Y,QUAN X,et al.Applying an electric field in a built-in zero valent iron---anaerobic reactor for enhancement of sludge granulation[J].Water Res,2011,45(3):1258-1266.
[36]XU X,LIN H,ZHU L,et al.Enhanced biodegradation of 2-chloronitro-benzene using a coupled zero-valent iron column and sequencing batch reactor system[J].J Chem Technol Biotechnol,2011,86(7):993-1000.
[37]ZHANG J,ZHANG Y,YANG L,et al.Enhancement of nitrogen removal in a novel anammox reactor packed with Fe electrode[J].Bioresour Technol,2012,114(3):102-108.
[38]KARRI S,SIERRAALVAREZ R,FIELD J A.Zero valent iron as an electron-donor for methanogenesis and sulfate reduction in anaerobic sludge[J].Biotechnol Bioeng,2005,92(7):810-819.
[39]马斌,张耀斌,全燮,等.ZVI强化厌氧处理高浓度颜料废水[J].环境工程学报,2015,9(2):767-772.
[40]徐浩,韩洪军,魏江波,等.零价铁强化上流式厌氧污泥床反应器处理煤化工费托合成废水研究[J].环境污染与防治,2017,39(8):845-850.
[41]刘轶文.零价铁强化厌氧废水处理的研究[D].大连:大连理工大学,2011.
[42]THRASH J C,COATES J D.Review:direct and indirect electrical stimulation of microbial metabolism[J].Environ Sci Technol,2008,42(11):3921-3931.
[43]SASAKI K,SASAKI D,MORITA M,et al.Bioelectrochemical system stabilizes methane fermentation from garbage slurry[J].Bioresour Technol,2010,101(10):3415-3422.
[44]NING X A,WEN W,ZHANG Y,et al.Enhanced dewaterability of textile dyeing sludge using micro-electrolysis pretreatment[J].J Environ Manage,2015,161:181-187.
[45]XIAO X,SHENG G P,MU Y,et al.A modeling approach to describe zvi-based anaerobic system[J].Water Res,2013,47(16):6007.
[46]OU C,SHEN J,ZHANG S,et al.Coupling of iron shavings into the anaerobic system for enhanced 2,4-dinitroanisole reduction in wastewater[J].Water Res,2016,101:457-466.
[47]WU D,ZHEN S,DING A,et al.Performance of a zero valent iron-based anaerobic system in swine wastewater treatment[J].JHazard Mater,2015,286:1-6.
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