煤化工废水中含氮杂环化合物处理研究进展
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摘要
含氮杂环化合物是煤化工废水中常见的有机污染物,是造成此类废水难于处理的主要原因之一。本文介绍了国内外对含氮杂环化合物处理的的生物方法和物理化学方法,总结了不同方法对含氮杂环化合物的降解途径、降解原理及降解效果,最后对煤化工废水中含氮杂环化合物的处理提出了进一步的研究方向。
Nitrogen heterocyclic compounds treatmentare are common organic pollutants in coal chemical industry wastewater,they are also the main reason that why this kind of wastewater is difficult to be treatment.The biological treatment methods and the physical and chemical processing method for nitrogen heterocyclic compounds at home and abroad were introduced in this paper,summarizes the degradation pathway,degradation principle and degradation effect of the nitrogen heterocyclic compounds by different methods,and finally the further research direction of nitrogen heterocyclic compounds in coal chemical industry wastewater treatment were proposed.
Nitrogen heterocyclic compounds treatmentare are common organic pollutants in coal chemical industry wastewater,they are also the main reason that why this kind of wastewater is difficult to be treatment.The biological treatment methods and the physical and chemical processing method for nitrogen heterocyclic compounds at home and abroad were introduced in this paper,summarizes the degradation pathway,degradation principle and degradation effect of the nitrogen heterocyclic compounds by different methods,and finally the further research direction of nitrogen heterocyclic compounds in coal chemical industry wastewater treatment were proposed.
引文
[1]金学文,李恩超,江一君,等.反渗透膜工艺用于焦化废水深度处理的实验研究[J].水处理技术,2014(4):59-62.
[2]Wei X X,Zhang Z Y,Fan Q L,et al.The effect of treatment stages on the coking wastewater hazardous compounds and their toxicity[J].Journal of Hazardous Materials,2012,23:135-141.
[3]孙丽娟,李咏梅,顾国维.含氮杂环化合物的生物降解研究进展[J].四川环境,2005,24(1):61-64.
[4]任大军.白腐菌对氮杂环化合物的降解及机理研究[D].武汉:华中科技大学,2006.
[5]Cui Zhao,Yin Zhang,Xiaobao Li,et al.Biodegradation of carbazole by the seven Pseudomonas sp.strains and their denitrification potential[J].Journal of Hazardous Materials,2011,190(1-3):253-259.
[6]Johanson S S,Licht D,Arvin E,et al.Metabolic pathway of quinoline,indole and their methylated analogs by Desulfobacteium indolicum(DSM 3383)[J].Appl Microbiol Biotechnol,1997,47:292-301.
[7]蔡晶晶.链霉菌(Streptomyces sp.)的筛选及其降解水中含氮杂环化合物的特性研究[D].杭州:浙江工商大学,2008.
[8]何苗,张晓健,瞿福平,等.杂环化合物及多环芳烃厌氧酸化降解性能的研究[J].中国给水排水,1997(3):13-16.
[9]Yang Hongwei,Jiang Zhanpeng,Shi Shaoqi.Biodegradability of nitrogenous compounds under anaerobic conditions and its estimation[J].Ecotoxicology&Environmental Safety,2006,63(2):299-305.
[10]蔡伊秋,程静,张超杰,等.氮杂环化合物2-甲基吡啶在缺氧条件下影响因素研究[J].水处理技术,2009,35(1):39-41.
[11]程静,蔡伊秋,张超杰,等.氮杂环化合物喹啉在缺氧条件下降解的影响因素[J].同济大学学报自然科学版,2009,37(9):1207-1211.
[12]郭少妮,金若菲,张爱丽,等.燃料灰吸附-再生处理氮杂环化合物废水的性能研究[J].环境工程,2014,32(2):41-44.
[13]程伟,高保娇,施雪军.功能接枝微粒PSSS/Si O2的制备及其对水介质中含氮杂环农药的吸附特性[J].环境化学,2013(3):402-409.
[14]许俊强,郭芳,全学军,等.焦化废水中的杂环化合物及多环芳烃降解的研究进展[J].化工进展,2008,27(7):973-976.
[15]Andreozzi R,Inzola A,Caprio A,et al.Quinoline ozonation in aqueous solution[J].Wat Res,1992,26:639-643.
[16]王小仛,黄霞,胡洪营.O3/UV降解喹啉过程中不同氧化剂的相对重要性[J].环境科学,2003,24(3):35-39.
[17]周莉,傅敏,肖洁,等.Ti O2光催化氧化焦化废水的实验研究[J].西南大学学报自然科学版,2007,29(7):59-63.
[18]Cocquet G,Ferroud C,Guy A.A mild and efficient procedure for ring-opening reactions of piperidine and pyrrolidine derivatives by single electron transfer photo oxidation[J].Etrahedron,2002,56:2975-2979.
[19]Allen D W,Clench M R,Morris J.Investigation of the products of oxidation of methylpyridines under aqueous conditions by gas chromatography-mass spectrometry[J].Analyst,1994,119:903-907.
[20]朱力思,黄正宏,温东辉,等.生物活性竹炭的制备及其对溶液中喹啉的去除[J].新型炭材料,2010,25(6):449-453.
[21]Padoley K V,Mudliar S N,Pandey R A.Heterocyclic nitrogenous pollutants in the environment and their treatment options-an overview[J].Bioresource Technology,2008,99(10):4029-4043.
[2]Wei X X,Zhang Z Y,Fan Q L,et al.The effect of treatment stages on the coking wastewater hazardous compounds and their toxicity[J].Journal of Hazardous Materials,2012,23:135-141.
[3]孙丽娟,李咏梅,顾国维.含氮杂环化合物的生物降解研究进展[J].四川环境,2005,24(1):61-64.
[4]任大军.白腐菌对氮杂环化合物的降解及机理研究[D].武汉:华中科技大学,2006.
[5]Cui Zhao,Yin Zhang,Xiaobao Li,et al.Biodegradation of carbazole by the seven Pseudomonas sp.strains and their denitrification potential[J].Journal of Hazardous Materials,2011,190(1-3):253-259.
[6]Johanson S S,Licht D,Arvin E,et al.Metabolic pathway of quinoline,indole and their methylated analogs by Desulfobacteium indolicum(DSM 3383)[J].Appl Microbiol Biotechnol,1997,47:292-301.
[7]蔡晶晶.链霉菌(Streptomyces sp.)的筛选及其降解水中含氮杂环化合物的特性研究[D].杭州:浙江工商大学,2008.
[8]何苗,张晓健,瞿福平,等.杂环化合物及多环芳烃厌氧酸化降解性能的研究[J].中国给水排水,1997(3):13-16.
[9]Yang Hongwei,Jiang Zhanpeng,Shi Shaoqi.Biodegradability of nitrogenous compounds under anaerobic conditions and its estimation[J].Ecotoxicology&Environmental Safety,2006,63(2):299-305.
[10]蔡伊秋,程静,张超杰,等.氮杂环化合物2-甲基吡啶在缺氧条件下影响因素研究[J].水处理技术,2009,35(1):39-41.
[11]程静,蔡伊秋,张超杰,等.氮杂环化合物喹啉在缺氧条件下降解的影响因素[J].同济大学学报自然科学版,2009,37(9):1207-1211.
[12]郭少妮,金若菲,张爱丽,等.燃料灰吸附-再生处理氮杂环化合物废水的性能研究[J].环境工程,2014,32(2):41-44.
[13]程伟,高保娇,施雪军.功能接枝微粒PSSS/Si O2的制备及其对水介质中含氮杂环农药的吸附特性[J].环境化学,2013(3):402-409.
[14]许俊强,郭芳,全学军,等.焦化废水中的杂环化合物及多环芳烃降解的研究进展[J].化工进展,2008,27(7):973-976.
[15]Andreozzi R,Inzola A,Caprio A,et al.Quinoline ozonation in aqueous solution[J].Wat Res,1992,26:639-643.
[16]王小仛,黄霞,胡洪营.O3/UV降解喹啉过程中不同氧化剂的相对重要性[J].环境科学,2003,24(3):35-39.
[17]周莉,傅敏,肖洁,等.Ti O2光催化氧化焦化废水的实验研究[J].西南大学学报自然科学版,2007,29(7):59-63.
[18]Cocquet G,Ferroud C,Guy A.A mild and efficient procedure for ring-opening reactions of piperidine and pyrrolidine derivatives by single electron transfer photo oxidation[J].Etrahedron,2002,56:2975-2979.
[19]Allen D W,Clench M R,Morris J.Investigation of the products of oxidation of methylpyridines under aqueous conditions by gas chromatography-mass spectrometry[J].Analyst,1994,119:903-907.
[20]朱力思,黄正宏,温东辉,等.生物活性竹炭的制备及其对溶液中喹啉的去除[J].新型炭材料,2010,25(6):449-453.
[21]Padoley K V,Mudliar S N,Pandey R A.Heterocyclic nitrogenous pollutants in the environment and their treatment options-an overview[J].Bioresource Technology,2008,99(10):4029-4043.
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