石墨烯基材料处理印染废水研究进
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摘要
石墨烯比表面积大,具备良好的化学稳定性,高吸附容量,在处理印染废水方面显示出巨大的优越性。介绍了石墨烯的结构和吸附印染废水的机理,重点讨论了石墨烯及其衍生物在处理印染废水方面的研究进展。最后对石墨烯基材料处理印染废水存在的问题和面临的挑战进行了总结和展望。
Graphene had large specific surface area, good chemical stability and high adsorption capacity.These properties made graphene become the most potential adsorption material for printing and dyeing wastewater. The structure of graphene and adsorption mechanism for printing and dyeing wastewater were introduced. The research progress of graphene and its derivatives in the treatment of printing and dyeing wastewater was emphatically discussed. Finally, the existing problems and challenges in the treatment of printing and dyeing wastewater by graphene-based materials were summarized and prospected.
Graphene had large specific surface area, good chemical stability and high adsorption capacity.These properties made graphene become the most potential adsorption material for printing and dyeing wastewater. The structure of graphene and adsorption mechanism for printing and dyeing wastewater were introduced. The research progress of graphene and its derivatives in the treatment of printing and dyeing wastewater was emphatically discussed. Finally, the existing problems and challenges in the treatment of printing and dyeing wastewater by graphene-based materials were summarized and prospected.
引文
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[25]马荣华,韩泽群.β3-SiW11Ni/氧化石墨烯复合材料的制备及对亚甲基蓝的吸附性能[J].化学试剂,2018,40(3):203-206.
[26]陈佳伟,赵一丹,杨利宁,等.石墨烯-Fe3O4@SiO2纳米复合材料去除水溶液中甲基红的研究[J].浙江师范大学学报:自然科学版,2018,41(2):68-73.
[27]姜丽丽,李传通,于海涛,等.石墨烯/碳纳米管复合材料的制备方法及应用进展[J].化学与生物工程,2017,34(2):1-5.
[2] CRINI G.Non-conventional low-cost adsorbents for dye removal:a review[J].Bioresource Technology,2006,97(9):1 061-1 085.
[3] SINGH K,ARORA S.Removal of synthetic textile dyes from wastewaters:a critical review on present treatment technologies[J].Critical Reviews in Environmental Science and Technology,2011,41(9):807-878.
[4] NOVOSELOV K S,GEIM A K,MOROZOV S V,et al.Electric field effect in atomically thin carbon films[J].Science,2004,306:666-669.
[5] WU Y A,YE F,SPELLER S,et al.Large single crystals of graphene on melted copper using chemical vapor deposition[J].Acs Nano,2012(6):5 010-5 017.
[6] YANG W,CHEN G R,SHI Z W,et al.Epitaxial growth of single-domain graphene on hexagonal boron nitride[J].Nat. Mater.,2013,12:792-797.
[7] PARK S,RUOFF R S.Chemical methods for the production of graphenes[J].Nat. Nanotechnol.,2009(4):217-224.
[8]庄媛,于飞,马杰,等.石墨烯去除水中重金属和抗生素的研究进展[J].功能材料,2014,45(23):23 001-23 009.
[9] SHAM A Y W,NOTLEY S M.Adsorption of organic dyes from aqueous solut ions using surfactant exfoliated graphene[J].J. Environ.Chem. Eng.,2018(6):495-504.
[10] LIU T,LI Y,DU Q,et al.Adsorption of methylene blue from aqueous solution by graphene[J].Colloids Surf. B Biointerfaces,2012,90(4):197-203.
[11] BRADDER P,LING S K,WANG S,et al.Dye adsorption on layered graphite oxide[J].J. Chem. Eng. Data,2010,56(1):138-141.
[12]武里鹏,刘淑娟,张伟强,等.新型三维立体结构氧化石墨烯材料的制备及其对亚甲基蓝的吸附[J].功能材料,2015,46(16):16 074-16 078.
[13] ZHAO G,WEN T,CHEN C,et al.Synthesis of graphene based nanomaterials and their application in energy related and environmental related areas[J].RSC Advances,2012,25(2):9 286-9 303.
[14] DREYER D R,PARK S,BIELAWSKI C,et al.The chemistry of graphene oxide[J].Chemical Society Reviews,2010,39(1):228-240.
[15]张倩,李可培,张惠云,等.三维石墨烯气凝胶的制备及对罗丹明B的吸附性能[J].印染,2018,44(10):1-7.
[16]刘怡虹,周廷尧,胡蓉,等.贻贝仿生三维石墨烯制备及对亚甲基蓝的吸附[J].环境化学,2018(11):1-7.
[17] WANG S,WEI J,LV S,et al.Removal of organic dyes in environmental water onto magnetic-sulfonic graphene nanocomposite[J].CleanSoil,Air,Water,2013,41(10):992-1 001.
[18]翟江丽,范亚.明胶改性磁性石墨烯对亚甲基蓝的吸附性能研究[J].分析科学学报,2018,34(4):539-543.
[19]张丽,罗汉金,方伟,等.改性氧化石墨烯/壳聚糖功能材料对刚果红的吸附研究[J].环境科学学报,2016,36(11):3 977-3 985.
[20] LERF A,HE H,FORSTER M,et al.Structure of graphite oxide revisited[J].J. Phys. Chem. B,1998,102(23):4 477-4 482.
[21] WU T,CAI X,TAN S,et al.Adsorption characteristics of acrylonitrile,p-toluenesulfonic acid,1-naphthalenesulfonic acid and methyl blue on graphene in aqueous solutions[J].Chemical Engineering Journal,2011,173(1):144-149.
[22] SUN H M,CAO L Y,LU L H.Magnetite/reduced graphene oxide nanocomposites:one step solvothermal synthesis and use as a novel platform for removal of dye pollutants[J].Nano Research,2011(4):550-562.
[23] RAMESHA G K, KUMARA A V, MURALIDHARA H B,et al.Graphene and grapheme oxide as effective adsorbents toward anionic and cationic dyes[J].Journal of Colloid and Interface Science,2011,361:270-277.
[24]曾会会,仪桂云,邢宝林,等.SiO2/还原氧化石墨烯复合材料的简易制备及对罗丹明B的吸附[J].化工进展,2018,37(3):1 084-1 091.
[25]马荣华,韩泽群.β3-SiW11Ni/氧化石墨烯复合材料的制备及对亚甲基蓝的吸附性能[J].化学试剂,2018,40(3):203-206.
[26]陈佳伟,赵一丹,杨利宁,等.石墨烯-Fe3O4@SiO2纳米复合材料去除水溶液中甲基红的研究[J].浙江师范大学学报:自然科学版,2018,41(2):68-73.
[27]姜丽丽,李传通,于海涛,等.石墨烯/碳纳米管复合材料的制备方法及应用进展[J].化学与生物工程,2017,34(2):1-5.