Nanoscale noble metals with a hollow interior formed through inside-out diffusion of silver in solid-state core-shell nanoparticles
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- 作者：Pengfei Hou (1) (2)
Penglei Cui (2)
Hui Liu (2)
Jianling Li (1)
Jun Yang (2)
1. State Key Laboratory of Advanced Metallurgy ; University of Science and Technology of Beijing ; 30 College Road ; Beijing ; 100083 ; China
2. State Key Laboratory of Multiphase Complex Systems ; Institute of Process Engineering ; Chinese Academy of Sciences ; Beijing ; 100190 ; China - 关键词：noble metal ; nanoparticle ; inside ; out diffusion ; solid ; state ; core ; shell ; hollow
- 刊名：Nano Research
- 出版年：2015
- 出版时间：February 2015
- 年：2015
- 卷：8
- 期：2
- 页码：512-522
- 全文大小：2,553 KB
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- 刊物主题：Chinese Library of Science
Chemistry
Nanotechnology - 出版者：Tsinghua University Press, co-published with Springer-Verlag GmbH
- ISSN：1998-0000
文摘
Noble metal nanoparticles with hollow interiors and customizable shell compositions have immense potential for a wide variety of applications. Herein, we present a facile, general, and cost-effective strategy for the synthesis of noble metal nanoparticles with hollow structures, which is based on the inside-out diffusion of Ag in solid-state core-shell nanoparticles. This approach starts with the preparation of core-shell nanoparticles with Ag residing in the core region, which are then loaded on a solid substrate and aged in air to allow the inside-out diffusion of Ag from the core region, leading to the formation of monometallic or alloy noble metal nanoparticles with a hollow interior. The synthesis was carried out at room temperature and could be achieved on different solid substrates. In particular, the inside-out diffusion of Ag calls for specific concern with respect to the evaluation of the catalytic performance of the Ag-based core-shell nanoparticles since it may potentially interfere with the physical and chemical properties of the core-shell particles.